Coal Geology & Exploration
Abstract
Objective This study aims to reveal the evolutionary patterns of reservoir parameters during the CO2-enhanced coalbed methane (CO2-ECBM) recovery and the impact of initial reservoir pressure on CBM recovery by gas injection. Methods Based on the multi-field coupling-based physical simulation experiment system of gas injection into coal seams for production growth, this study conducted experiments of CH4 displacement by CO2 under a constant gas injection pressure of 2.0 MPa and initial reservoir pressures of 1.5 MPa, 1.0 MPa, and 0.5 MPa. Accordingly, this study explored the spatiotemporal evolutionary patterns of multiphysical field parameters such as reservoir pressure, temperature, and volumetric strain during CH4 displacement by CO2, as well as the displacement effects. Moreover, this study divided the displacement process into three stages (i.e., stages 1, 2, and 3) by analyzing the interaction mechanisms. Results and Conclusions The results indicate that in the displacement process, the reservoir pressure in the injection well was higher than that in the production well. Their pressure difference increased with the initial reservoir pressure, with a maximum of 0.34 MPa. In contrast, the reservoir equilibrium pressure decreased with an increase in the initial reservoir pressure. The reservoir temperature rose earlier at a location closer to the injection well, and it rose at a higher rate under a lower initial reservoir pressure. Furthermore, the reservoir equilibrium temperature decreased with an increase in the initial reservoir pressure. The evolutionary process of reservoir volumetric strain was divided into three stages: slow increase, rapid increase, and stabilization, and the reservoir volumetric strain decreased with an increase in the initial reservoir pressure. During the displacement, as the initial reservoir pressure increased from 0.5 MPa to 1.0 MPa and then to 1.5 MPa, the CH4 recovery decreased from 91.00 % to 88.48 % and then to 86.81 %, showing a decreasing trend with increasing initial reservoir pressure. In contrast, the CO2 breakthrough time and CO2 storage efficiency increased with the initial reservoir pressure. The displacement process exhibited varying mechanisms in various stages. In stage 1 (CO2 pre-breakthrough stage) and stage 2 (CO2 breakthrough stage), the cumulative CH4 volume and CO2 storage capacity increased with the initial reservoir pressure, both representing over 80 % of the corresponding total volumes of the whole displacement process. The results of this study provide a theoretical basis for developing an integrated technology for efficient CBM recovery and CO2 geological storage.
Keywords
CO2-ECBM, initial reservoir pressure, reservoir parameters evolution, displacement effect, multi-field coupling, true three-axis stress state
DOI
10.12363/issn.1001-1986.24.12.0798
Recommended Citation
XU Jiang, JIANG Shiyu, PENG Shoujian,
et al.
(2025)
"An experimental study of CH4 displacement by CO2 under varying initial reservoir pressures,"
Coal Geology & Exploration: Vol. 53:
Iss.
4, Article 9.
DOI: 10.12363/issn.1001-1986.24.12.0798
Available at:
https://cge.researchcommons.org/journal/vol53/iss4/9
Reference
[1] 王国法. 煤矿智能化最新技术进展与问题探讨[J]. 煤炭科学技术,2022,50(1):1−27.
WANG Guofa. New technological progress of coal mine intelligence and its problems[J]. Coal Science and Technology,2022,50(1):1−27.
[2] 徐凤银,侯伟,熊先钺,等. 中国煤层气产业现状与发展战略[J]. 石油勘探与开发,2023,50(4):669−682.
XU Fengyin,HOU Wei,XIONG Xianyue,et al. The status and development strategy of coalbed methane industry in China[J]. Petroleum Exploration and Development,2023,50(4):669−682.
[3] 姚艳斌,孙晓晓,万磊. 煤层CO2地质封存的微观机理研究[J]. 煤田地质与勘探,2023,51(2):146−157.
YAO Yanbin,SUN Xiaoxiao,WAN Lei. Micro–mechanism of geological sequestration of CO2 in coal seam[J]. Coal Geology & Exploration,2023,51(2):146−157.
[4] 桑树勋,袁亮,刘世奇,等. 碳中和地质技术及其煤炭低碳化应用前瞻[J]. 煤炭学报,2022,47(4):1430−1451.
SANG Shuxun,YUAN Liang,LIU Shiqi,et al. Geological technology for carbon neutrality and its application prospect for low carbon coal exploitation and utilization[J]. Journal of China Coal Society,2022,47(4):1430−1451.
[5] 肖智勇,王刚,刘杰,等. 热–流–固耦合作用下含水煤层渗透率模型建立及应用研究[J]. 岩石力学与工程学报,2024,43(12):3044−3057.
XIAO Zhiyong,WANG Gang,LIU Jie,et al. A permeability model of water–bearing coal seams under thermo–hydro–mechanical coupling effect and its application[J]. Chinese Journal of Rock Mechanics and Engineering,2024,43(12):3044−3057.
[6] 刘世奇,皇凡生,杜瑞斌,等. CO2地质封存与利用示范工程进展及典型案例分析[J]. 煤田地质与勘探,2023,51(2):158−174.
LIU Shiqi,HUANG Fansheng,DU Ruibin,et al. Progress and typical case analysis of demonstration projects of the geological sequestration and utilization of CO2[J]. Coal Geology & Exploration,2023,51(2):158−174.
[7] VAN BERGEN F,KRZYSTOLIK P,VAN WAGENINGEN N,et al. Production of gas from coal seams in the Upper Silesian Coal Basin in Poland in the post–injection period of an ECBM pilot site[J]. International Journal of Coal Geology,2009,77(1/2):175−187.
[8] 黄中伟,李国富,杨睿月,等. 我国煤层气开发技术现状与发展趋势[J]. 煤炭学报,2022,47(9):3212−3238.
HUANG Zhongwei,LI Guofu,YANG Ruiyue,et al. Review and development trends of coalbed methane exploitation technology in China[J]. Journal of China Coal Society,2022,47(9):3212−3238.
[9] 桑树勋. 二氧化碳地质存储与煤层气强化开发有效性研究述评[J]. 煤田地质与勘探,2018,46(5):1−9.
SANG Shuxun. Research review on technical effectiveness of CO2 geological storage and enhanced coalbed methane recovery[J]. Coal Geology & Exploration,2018,46(5):1−9.
[10] 张松航,唐书恒,张守仁,等. 不同排采程度煤储层注CO2驱煤层气模拟评价[J]. 煤炭学报,2022,47(3):1275−1285.
ZHANG Songhang,TANG Shuheng,ZHANG Shouren,et al. Simulation and evaluation of enhanced coalbed methane recovery by CO2 storage in coal reservoirs with different drainage and production levels[J]. Journal of China Coal Society,2022,47(3):1275−1285.
[11] TANG Jun,LONG Yonghan,ZHANG Lei,et al. Experimental study of coal rank effect on carbon dioxide injection to enhance CBM recovery[J]. Fuel,2023,354:129393.
[12] 孙泽东,任泫琦. 超临界CO2对烟煤Ⅰ型断裂韧性影响的实验研究[J]. 中国煤炭,2024,50(9):99−110.
SUN Zedong,REN Xuanqi. Experimental study on the effect of supercritical CO2 on bituminous coal type Ⅰ fracture toughness[J]. China Coal,2024,50(9):99−110.
[13] LIU Shiqi,WANG He,SANG Shuxun,et al. Effects of pore structure changes on the CH4 adsorption capacity of coal during CO2–ECBM[J]. Fuel,2022,330:125529.
[14] 王建美,梁卫国,牛栋,等. 超临界CO2作用下无烟煤结构响应及高压吸附机理[J/OL]. 天然气工业,2024:1–13 [2024-03-20]. http://kns.cnki.net/KCMS/detail/detail.aspx?filename=TRQG20240314001&dbname=CJFD&dbcode=CJFQ.
WANG Jianmei,LIANG Weiguo,NIU Dong,et al. Study on the structural response and adsorption mechanism of anthracite coal with supercritical CO2 effects[J/OL]. Natural Gas Industry,2024:1–13 [2024-03-20]. http://kns.cnki.net/KCMS/detail/detail.aspx?filename=TRQG20240314001&dbname=CJFD&dbcode=CJFQ.
[15] 周西华,韩明旭,白刚,等. CO2注气压力对瓦斯扩散系数影响规律实验研究[J]. 煤田地质与勘探,2021,49(1):81−86.
ZHOU Xihua,HAN Mingxu,BAI Gang,et al. Experimental study on the influence of CO2 injection pressure on gas diffusion coefficient[J]. Coal Geology & Exploration,2021,49(1):81−86.
[16] 韩光,付志豪,白刚,等. CO2注气压力对CH4驱替特性影响实验研究[J]. 中国安全生产科学技术,2022,18(8):85−90.
HAN Guang,FU Zhihao,BAI Gang,et al. Experimental study on influence of CO2 injection pressure on CH4 displacement characteristics[J]. Journal of Safety Science and Technology,2022,18(8):85−90.
[17] 姜延航,白刚,周西华,等. 煤层注CO2驱替CH4影响因素试验研究[J]. 中国安全科学学报,2022,32(4):113−121.
JIANG Yanhang,BAI Gang,ZHOU Xihua,et al. Experimental study on influence factors of CH4 displacement by CO2[J]. China Safety Science Journal,2022,32(4):113−121.
[18] 白刚,姜延航,周西华,等. 不同CO2注入温度置换驱替CH4特性试验研究[J]. 煤炭科学技术,2021,49(5):167−174.
BAI Gang,JIANG Yanhang,ZHOU Xihua,et al. Experimental study on characteristics of replacement and displacement of CH4 at different CO2 injection temperatures[J]. Coal Science and Technology,2021,49(5):167−174.
[19] BAI Gang,SU Jun,LI Xueming,et al. Step–by–step CO2 injection pressure for enhanced coal seam gas recovery:A laboratory study[J]. Energy,2022,260:125197.
[20] 梁卫国,吴迪,赵阳升. CO2驱替煤层CH4试验研究[J]. 岩石力学与工程学报,2010,29(4):665−673.
LIANG Weiguo,WU Di,ZHAO Yangsheng. Experimental study of coalbeds methane replacement by carbon dioxide[J]. Chinese Journal of Rock Mechanics and Engineering,2010,29(4):665−673.
[21] 桑树勋,牛庆合,曹丽文,等. 深部煤层CO2注入煤岩力学响应特征及机理研究进展[J]. 地球科学,2022,47(5):1849−1864.
SANG Shuxun,NIU Qinghe,CAO Liwen,et al. Mechanical response characteristics and mechanism of coal–rock with CO2 injection in deep coal seam:A review[J]. Earth Science,2022,47(5):1849−1864.
[22] LIU Zhengdong,CHENG Yuanping,WANG Yongkang,et al. Experimental investigation of CO2 injection into coal seam reservoir at in–situ stress conditions for enhanced coalbed methane recovery[J]. Fuel,2019,236:709−716.
[23] BAI Gang,SU Jun,ZHANG Zunguo,et al. Effect of CO2 injection on CH4 desorption rate in poor permeability coal seams:An experimental study[J]. Energy,2022,238:121674.
[24] 杨天鸿,陈立伟,杨宏民,等. 注二氧化碳促排煤层瓦斯机制转化过程实验研究[J]. 东北大学学报(自然科学版),2020,41(5):623−628.
YANG Tianhong,CHEN Liwei,YANG Hongmin,et al. Experimental study on the conversion process of promoting gas drainage mechanism by CO2 injection[J]. Journal of Northeastern University(Natural Science),2020,41(5):623−628.
[25] LI Zhenbao,WANG Shaorui,WEI Gaoming,et al. The seepage driving mechanism and effect of CO2 displacing CH4 in coal seam under different pressures[J]. Energy,2024,293:130740.
[26] JIA Li,PENG Shoujian,XU Jiang,et al. Experimental investigation on disturbance effect during coalbed methane production[J]. Journal of Petroleum Science and Engineering,2022,208:109591.
[27] ZHANG Chaolin,WANG Enyuan,LI Bobo,et al. Laboratory experiments of CO2–enhanced coalbed methane recovery considering CO2 sequestration in a coal seam[J]. Energy,2023,262:125473.
[28] PAN Zhejun,YE Jianping,ZHOU Fubao,et al. CO2 storage in coal to enhance coalbed methane recovery:A review of field experiments in China[J]. International Geology Review,2018,60(5/6):754−776.
[29] LI Qixian,XU Jiang,PENG Shoujian,et al. Dynamic evolution of the fluid effect of multiple reservoirs due to CBM coproduction:An experimental investigation[J]. Energy & Fuels,2020,34(9):10947−10957.
[30] 高彩霞,禹艺娜,李志军,等. 高、低阶煤孔隙结构差异性及其对甲烷吸附特性的影响研究[J]. 中国煤炭,2024,50(5):113−119.
GAO Caixia,YU Yina,LI Zhijun,et al. Research on the difference of pore structure between high and low rank coal and its influence on methane adsorption characteristics[J]. China Coal,2024,50(5):113−119.
[31] WANG Zhonghui,LI Bobo,REN Chonghong,et al. Energy–driven damage constitutive model of water–bearing coal under triaxial compression[J]. Rock Mechanics and Rock Engineering,2024,57(2):1309−1328.
[32] JIA Li,PENG Shoujian,XU Jiang,et al. Investigation on gas drainage effect under different borehole layout via 3D monitoring of gas pressure[J]. Journal of Natural Gas Science and Engineering,2022,101:104522.
[33] 范晶晶. 煤层CO2封存影响因素及数值模拟研究[D]. 北京:中国矿业大学(北京),2018.
FAN Jingjing. Research on the influence factors of CO2 sequestration in coal seams and numerical simulation of CO2 sequestration process[D]. Beijing:China University of Mining & Technology(Beijing),2018.
[34] XU Jizhao,QIAN Sheng,XU Hexiang,et al. Numerical analysis of reservoir features and injection modes on carbon exchange capacity during CO2–ECBM processes[J]. Energy & Fuels,2024,38(21):20485−20503.
[35] 王飞,邢好运,李万春,等. 中低阶煤的孔隙结构演化特征[J]. 西安科技大学学报,2020,40(3):384−392.
WANG Fei,XING Haoyun,LI Wanchun,et al. Evolution characteristics of pore structure in medium and low rank coal[J]. Journal of Xi’an University of Science and Technology,2020,40(3):384−392.
[36] WANG Zhonghui,LI Bobo,REN Chonghong,et al. A permeability model for coal based on elastic and plastic deformation conditions under the interaction of hydro–mechanical effects[J]. Journal of Petroleum Science and Engineering,2022,212:110209.
[37] SU Erlei,WEI Jiaqi,CHEN Haidong,et al. Effect of CO2 injection on coalbed permeability based on a thermal–hydraulic–mechanical coupling model[J]. Energy & Fuels,2024,38(12):11078−11092.
Included in
Earth Sciences Commons, Mining Engineering Commons, Oil, Gas, and Energy Commons, Sustainability Commons